Our theme

With applications ranging from high-resolution sensing to quantum information science, spin control at the nanoscale is emerging as an area of newfound importance. Specific topics of interest guiding our research effort are (i) the development of new spin-based platforms for nanometer-resolution MRI and various nanoscale sensing protocols, (ii) quantum control of individual spin clusters for quantum information processing, and (iii) the generation of electron or nuclear spin hyper-polarization. We are presently inviting applications for a POSTDOCTORAL POSITION in our group. To learn more please click here.

To guide you through our website we have assembled a set of short movies describing some conceptual and practical aspects of our work. An intro video clip by Prof. Meriles follows below.

We are conducting a range of experiments centered on the understanding and manipulation of individual or small ensembles of paramagnetic defects. Illustrative examples along with more images and video clips can be found in our Research page. We also suggest you check out these recent Publications:

“Long-term spin state storage using ancilla charge memories”, H. Jayakumar,  A. Lozovoi, D. Daw, C.A. Meriles, submitted. Available as arXiv:2003.13148.

“Optically pumped spin polarization as a probe of many-body thermalization”, D. Pagliero, P. Zangara, J. Henshaw, A. Ajoy, R.H. Acosta, J.A. Reimer, A. Pines, C.A. Meriles, Science Adv. 6, eaaz6986 (2020).  Available as arXiv:2005.00647.

“Mechanical rotation via optical pumping of paramagnetic impurities”, P.R. Zangara, A. Wood, M.W. Doherty, C.A. Meriles, Phys. Rev. B 100, 235410 (2019). Available as arXiv:1912.03524.

13C dynamic nuclear polarization in diamond via a microwave-free ‘integrated’ cross effect”, J. Henshaw, D. Pagliero, P.R. Zangara, B. Franzoni, A. Ajoy, R. Acosta, J.A. Reimer, A. Pines, C.A. Meriles, Proc. Natl. Acad. Sci. USA 116, 18334 (2019). Available as arXiv:1909.06642.

“Scalable microcavity-coupled quantum emitters in 2D hexagonal boron nitride”, N.V. Proscia, H. Jayakumar, X. Ge, G.l. Lopez-Morales, Z. Shotan, W. Zhou, C.A. Meriles, V.M. Menon, Nanophotin pressAvailable as arXiv:1906.06546.

“Hyperpolarized relaxometry based nuclear T1 noise spectroscopy in hybrid diamond quantum registers”, A. Ajoy, B. Safvati, R. Nazaryan, J.T. Oon, B. Han, P. Raghavan, R. Nirodi, A. Aguilar, K. Liu, X. Cai, X. Lv, E. Druga, C. Ramanathan, J.A. Reimer, C.A. Meriles, D. Suter, A. Pines, Nature Commun. 10, 5160 (2019). Available as arXiv:1902.06204.

“Dynamics of frequency-swept nuclear spin optical pumping in powdered diamond at low magnetic fields”, P.R. Zangara, S. Dhomkar, A. Ajoy, K. Liu, R. Nazarian, D. Pagliero, D. Suter, J.A. Reimer, A. Pines, C.A. Meriles, Proc. Natl. Acad. Sci. USA 116, 2512 (2019)Available as arXiv:1902.06805.

“Near-deterministic activation of single-photon emitters in hexagonal boron nitride”, N. Proscia, Z. Shotan, H. Jayakumar, P. Reddy, M. Dollar, A. Alkauskas, M.W. Doherty, C.A. Meriles, V.M. Menon, Optica 5, 1128 (2018). Available  as arXiv:1712.01352.

“Orientation independent room-temperature optical 13C hyperpolarization in powdered diamond”, A. Ajoy, K. Liu, R. Nazaryan, X. Lv, P.R. Zangara, B. Safvati, G. Wang, D. Arnold, G. Li, A. Lin, P. Raghavan, E. Druga, S. Dhomkar, D. Pagliero, J.A. Reimer, D. Suter, C.A. Meriles, A. Pines, Science Adv. 4, eaar5492 (2018).

“Charge dynamics in near-surface, variable-density ensembles of nitrogen-vacancy centers in diamond”, S. Dhomkar, H. Jayakumar, P.R. Zangara, C.A. Meriles, Nano Lett. 18, 4046 (2018). (ASAP article). Available as arXiv:1807.00229.

“Microwave-assisted cross-polarization of nuclear spin ensembles from optically-pumped nitrogen-vacancy centers in diamond”, F. Shagieva, S. Zaiser, P. Neumann, D.B.R. Dasari, R. Stöhr, A. Denisenko, R. Reuter, C.A. Meriles, J. Wrachtrup, Nano Lett. 18, 3731 (2018).  (ASAP article). Available as arXiv:1803.05608v1.

“On-demand generation of neutral and negatively-charged silicon-vacancy centers in diamond”, S. Dhomkar, P. Zangara, C.A. Meriles, Phys. Rev. Lett. 120, 117401 (2018). Available as arXiv:1803.06569v1.

“Non-volatile nuclear spin memory enables sensor-unlimited nanoscale spectroscopy of small spin clusters”, M. Pfender, N. Aslam, H. Sumiya, S. Onoda, P. Neumann, J. Isoya, C.A. Meriles, J. Wrachtrup, Nature Commun. 8, 834 (2017). Available as arXiv:1610.05675.

“Photo-induced modification of single photon emitters in hexagonal boron nitride”, Z. Shotan, H. Jayakumar, C.R. Considine, M. Mackoit, H. Fedder, J. Wrachtrup, A. Alkauskas, M.W. Doherty, V.M. Menon, C.A. Meriles, ACS Photonics 3, 2490 (2016).

“Long-term data storage in diamond”, S. Dhomkar, J. Henshaw, H. Jayakumar, C.A. Meriles, Science Adv. 2, e1600911 (2016). Available as arXiv:1610.09022.

“Optical patterning of trapped charge in nitrogen-doped diamond”, H. Jayakumar, J. Henshaw, S. Dhomkar, D. Pagliero, A. Laraoui, N.B. Manson, R. Albu, M.W. Doherty, C.A.. Meriles, Nature Commun. 7, 12660 (2016). Available as arXiv:1609.03085.

“Towards a room-temperature spin quantum bus in diamond via optical spin injection, transport and detection”, M.W. Doherty, C.A. Meriles, A. Alkauskas, H. Fedder, M.J. Sellars, N.B. Manson, Phys. Rev. X 6, 041035 (2016). Available as arXiv:1511.08559.

“Imaging thermal conductivity with nanoscale resolution using a scanning spin probe”, A. Laraoui, H. Aycock-Rizzo, X. Lu, Y. Gao, E. Riedo, C.A. Meriles, Nature Commun. 6, 8954 (2015)Available as arXiv:1511.06916.

“Probing molecular dynamics at the nanoscale via an individual paramagnetic center”, T.M. Staudacher, N. Raatz, S. Pezzagna, J. Meijer, F. Reinhard, C.A. Meriles, J. Wrachtrup, Nature Commun. 6, 8527 (2015).  Available as arXiv:1507.05921.

“Dynamic nuclear spin polarization of liquids and gases in contact with nanostructured diamond”, D. Abrams, M.E. Trusheim, D. Englund, M.D. Shattuck, C.A. Meriles, Nano Lett. 14, 2471 (2014).

“Scalable Fabrication of High Purity Diamond Nanocrystals with Long-Spin-Coherence Nitrogen Vacancy Centers”, M. E. Trusheim, L. Li, A. Laraoui, E.H. Chen, O. Gaathon, H. Bakhru, T. Schroeder, C.A. Meriles, D. Englund, Nano Lett. 14, 32 (2014). 

“Approach to dark spin cooling in a diamond nanocrystal”, A. Laraoui, C.A. Meriles, ACS Nano 7, 3403 (2013).

“High-Resolution Correlation Spectroscopy of 13C Spins Near a Nitrogen-Vacancy Center in Diamond”, A. Laraoui, F. Dolde, C. Burk, F. Reinhard, J. Wrachtrup, C.A. Meriles, Nature Commun. 4, 1651 (2013). Available as arXiv:1305.1536.

“Nuclear magnetic resonance spectroscopy on a (5nm)^3 volume of liquid and solid samples”, T. Staudacher, F. Shi, S. Pezzagna, J. Meijer, J. Du, C.A. Meriles, F. Reinhard, J. Wrachtrup, Science 339, 561 (2013).

“Nitrogen-Vacancy-assisted magnetometry of paramagnetic centers in an individual diamond nanocrystal” A. Laraoui, J.S. Hodges, C.A. Meriles, Nano Lett. 12, 3477 (2012).

“Optically re-writable patterns of nuclear magnetization in Gallium Arsenide”, J.P. King, Y. Li, L. C.A. Meriles, J.A. Reimer, Nature Commun. 3, 918 (2012). 

Our laboratories are located at the Center for Discovery and Innovation (CDI), part of a new science complex on the CCNY campus. Also part of this initiative is the CUNY Advanced Science Research Center (ASRC), a state-of-the-art cross-disciplinary facility housing the most advanced nanofab in the New York area. Check out the photos below or take our Virtual Tour to learn more!